Exciton-exciton annihilation

A new study led by C. Heshmatpour and J. Hauer from TU München studies exciton-exciton annihilation in a squaraine trimer. The experiment exploits 5th-order optical spectroscopy to study the evolution of the trimer after two-photon excitation into its bi-exciton state. Quantum chemistry computations performed by M. Menger, now located at Groningen, provide the required parameters to model the experimental signals within a Frenkel exciton model. The associated article Annihilation Dynamics of Molecular Excitons Measured at a Single Perturbative Excitation Energy just appeared in J. Phys. Chem. Lett.

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